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["Cu2O/Cu",null,"CuO@Cu"]
["2θ (degree)","Intensity (arb. units)","2θ (degree)","Intensity (arb. units)"]
[5,582,5,581]
[5.02046,627,5.02046,636]
[5.04093,633,5.04093,579]
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{"sheet":"Fig1c","index":1,"n_rows":253,"n_cols":4,"rows_kept":253,"merged":[[0,0,0,1],[0,2,0,3]]}
["initial",null,"After CV activation"]
["Kinetic energy (eV)","Intensity (arb. units)","Kinetic energy (eV)","Intensity (arb. units)"]
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{"sheet":"Fig1d","index":2,"n_rows":1017,"n_cols":4,"rows_kept":1017,"merged":[[0,0,0,1],[0,2,0,3]]}
["Initial",null,"After CV activation"]
["Raman Shift (cm-1)","Intensity (arb. units)","Raman Shift (cm-1)","Intensity (arb. units)"]
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[165.229,4071.26,165.229,77.3514]
[163.289,4132.26,163.289,83.7795]
[161.349,4135.25,161.349,79.8957]
[159.409,4218.11,159.409,72.1485]
[157.468,4321.55,157.468,78.5737]
[155.527,4339.95,155.527,66.9666]
[153.585,4408.56,153.585,70.815]
[151.643,4432.08,151.643,72.0873]
[149.7,4589.44,149.7,74.646]
[147.757,4718.43,147.757,75.9169]
[145.814,4665.97,145.814,79.7602]
[143.87,4667.56,143.87,78.4572]
[141.926,4651.14,141.926,75.8688]
[139.982,4602.59,139.982,82.281]
[138.037,4578.49,138.037,70.6954]
[136.091,4571.1,136.091,89.957]
[134.145,4678.06,134.145,69.3808]
[132.199,4723.33,132.199,82.2118]
[130.253,4723.62,130.253,75.7731]
[128.306,4750.88,128.306,82.1773]
[126.358,4760.15,126.358,75.7414]
[124.41,4979.91,124.41,84.7099]
[122.462,4973.74,122.462,75.7097]
[120.514,5156.16,120.514,76.9768]
[118.565,5368.01,118.565,76.9608]
[116.615,5623.38,116.615,79.5095]
[114.665,5651.7,114.665,80.7751]
[112.715,5854.34,112.715,73.0671]
[110.764,6017.17,110.764,93.5577]
[108.813,6064.61,108.813,90.9756]
[106.862,6222.21,106.862,89.6756]
[104.91,6320.82,104.91,76.8489]
[102.958,6546.17,102.958,76.833]
[101.005,6528.18,101.005,74.2566]
[99.0518,6484.59,99.0518,83.2014]
[97.0983,6636.82,97.0983,83.1842]
[95.1444,6634.18,95.1444,88.2851]
[93.1901,6508.73,93.1901,92.1046]
[91.2354,6524.02,91.2354,81.8539]
[89.2803,6255.43,89.2803,67.7714]
[87.3248,6131.41,87.3248,84.3772]
[85.3689,5979.33,85.3689,92.0291]
[83.4126,5819.65,83.4126,88.1765]
[81.4559,5629.36,81.4559,81.7702]
[79.4988,5570.73,79.4988,90.6953]
[77.5413,5325.66,77.5413,86.8453]
[75.5834,5213.49,75.5834,100.873]
[73.6251,5038.81,73.6251,91.9165]
[71.6664,4794,71.6664,82.9633]
[69.7073,4629.69,69.7073,68.9094]
[67.7478,4410.58,67.7478,93.1364]
[65.7879,4467.09,65.7879,81.6373]
[63.8276,4382.01,63.8276,76.5195]
[61.8669,4337.78,61.8669,91.8048]
[59.9058,4107.44,59.9058,87.9619]

{"sheet":"Fig1g","index":3,"n_rows":6,"n_cols":2,"rows_kept":6}
[null,"Cu concentration (mg L-1)"]
["1 cycle",0.528]
["5 cycle",0.663]
["10 cycle",0.472]
["50 cycle",0.133]
["100 cycle",0.011]

{"sheet":"Fig2a","index":4,"n_rows":1002,"n_cols":6,"rows_kept":1002,"merged":[[0,0,0,1],[0,2,0,3],[0,4,0,5]]}
["Cu foam",null,"CuO@Cu",null,"OD-Cu"]
["Potential (V) vs. RHE","Current density (A cm-2)","Potential (V) vs. RHE","Current density (A cm-2)","Potential (V) vs. RHE","Current density (A cm-2)"]
[0.03725,{"v":-1.917E-4,"d":"-1.92E-04"},0.13461,0.00187,0.23,{"v":0.0007671,"d":"7.67E-04"}]
[0.03626,{"v":-2.065E-4,"d":"-2.07E-04"},0.13405,0.00152,0.229,{"v":0.0004558,"d":"4.56E-04"}]
[0.03527,{"v":-2.117E-4,"d":"-2.12E-04"},0.1334,1.25E-3,0.228,{"v":0.000289,"d":"2.89E-04"}]
[0.03427,{"v":-0.0002093,"d":"-2.09E-04"},0.13267,0.00104,0.227,{"v":0.0001723,"d":"1.72E-04"}]
[0.03327,{"v":-2.119E-4,"d":"-2.12E-04"},0.13189,{"v":0.0008708,"d":"8.71E-04"},0.226,{"v":9.78e-05,"d":"9.78E-05"}]
[0.03227,{"v":-0.0002124,"d":"-2.12E-04"},0.13107,{"v":0.0007268,"d":"7.27E-04"},0.225,{"v":4.006e-05,"d":"4.01E-05"}]
[0.03128,{"v":-0.0002188,"d":"-2.19E-04"},0.13023,{"v":0.0006052,"d":"6.05E-04"},0.224,{"v":-2.16E-5,"d":"-2.16E-05"}]
[0.03028,{"v":-0.000218,"d":"-2.18E-04"},0.12936,{"v":0.0005034,"d":"5.03E-04"},0.223,{"v":-7.973e-05,"d":"-7.97E-05"}]
[0.02928,{"v":-0.0002171,"d":"-2.17E-04"},0.12847,{"v":0.0004114,"d":"4.11E-04"},0.222,{"v":-0.0001274,"d":"-1.27E-04"}]
[0.02828,{"v":-0.000217,"d":"-2.17E-04"},0.12757,{"v":3.321E-4,"d":"3.32E-04"},0.221,{"v":-0.0001575,"d":"-1.58E-04"}]
[0.02728,{"v":-0.0002212,"d":"-2.21E-04"},0.12667,{"v":2.586E-4,"d":"2.59E-04"},0.22,{"v":-0.0001843,"d":"-1.84E-04"}]
[0.02628,{"v":-0.000221,"d":"-2.21E-04"},0.12576,{"v":0.0001913,"d":"1.91E-04"},0.219,{"v":-0.0002172,"d":"-2.17E-04"}]
[0.02528,{"v":-2.196E-4,"d":"-2.20E-04"},0.12484,{"v":0.0001286,"d":"1.29E-04"},0.218,{"v":-0.000254,"d":"-2.54E-04"}]
[0.02428,{"v":-2.187E-4,"d":"-2.19E-04"},0.12392,{"v":6.52e-05,"d":"6.52E-05"},0.217,{"v":-0.0002891,"d":"-2.89E-04"}]
[0.02329,{"v":-2.243E-4,"d":"-2.24E-04"},0.12299,{"v":1.155E-5,"d":"1.16E-05"},0.216,{"v":-0.0003151,"d":"-3.15E-04"}]
[0.02229,{"v":-0.0002282,"d":"-2.28E-04"},0.12205,{"v":-3.653e-05,"d":"-3.65E-05"},0.215,{"v":-0.000332,"d":"-3.32E-04"}]
[0.02129,{"v":-0.000228,"d":"-2.28E-04"},0.1211,{"v":-8.185e-05,"d":"-8.19E-05"},0.214,{"v":-3.457E-4,"d":"-3.46E-04"}]
[0.0203,{"v":-0.0002305,"d":"-2.31E-04"},0.12015,{"v":-1.193E-4,"d":"-1.19E-04"},0.213,{"v":-0.0003668,"d":"-3.67E-04"}]
[0.01928,{"v":-2.218E-4,"d":"-2.22E-04"},0.1192,{"v":-0.0001581,"d":"-1.58E-04"},0.212,{"v":-0.0003945,"d":"-3.95E-04"}]
[0.01828,{"v":-0.0002183,"d":"-2.18E-04"},0.11825,{"v":-1.942E-4,"d":"-1.94E-04"},0.211,{"v":-4.238E-4,"d":"-4.24E-04"}]
[0.01728,{"v":-0.0002222,"d":"-2.22E-04"},0.11729,{"v":-0.00023,"d":"-2.30E-04"},0.21,{"v":-0.0004346,"d":"-4.35E-04"}]
[0.01628,{"v":-0.0002204,"d":"-2.20E-04"},0.11634,{"v":-0.0002666,"d":"-2.67E-04"},0.209,{"v":-0.0004419,"d":"-4.42E-04"}]
[0.01528,{"v":-0.0002183,"d":"-2.18E-04"},0.11538,{"v":-0.0002985,"d":"-2.99E-04"},0.208,{"v":-0.000454,"d":"-4.54E-04"}]
[0.01428,{"v":-2.206E-4,"d":"-2.21E-04"},0.11442,{"v":-3.302E-4,"d":"-3.30E-04"},0.207,{"v":-0.0004806,"d":"-4.81E-04"}]
[0.01329,{"v":-2.265E-4,"d":"-2.27E-04"},0.11346,{"v":-0.0003617,"d":"-3.62E-04"},0.206,{"v":-0.0004998,"d":"-5.00E-04"}]
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[0.01129,{"v":-0.0002279,"d":"-2.28E-04"},0.11154,{"v":-0.0004185,"d":"-4.19E-04"},0.204,{"v":-0.0005159,"d":"-5.16E-04"}]
[0.01029,{"v":-0.0002272,"d":"-2.27E-04"},0.11057,{"v":-0.0004432,"d":"-4.43E-04"},0.203,{"v":-0.0005164,"d":"-5.16E-04"}]
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[3.3E-3,{"v":-0.0002382,"d":"-2.38E-04"},0.10375,{"v":-0.0005852,"d":"-5.85E-04"},0.196,{"v":-0.000606,"d":"-6.06E-04"}]
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[1.31E-3,{"v":-0.0002435,"d":"-2.44E-04"},0.1018,{"v":-0.0006224,"d":"-6.22E-04"},0.194,{"v":-6.2E-4,"d":"-6.20E-04"}]
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["Scanning rate (mV s-1)","Current density (mA cm-2)","Scanning rate (mV s-1)","Current density (mA cm-2)","Scanning rate (mV s-1)","Current density (mA cm-2)"]
[100,4.3,100,5,100,4.6]
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[60,2.955,60,3.46,60,3.183]
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{"sheet":"Fig2d","index":7,"n_rows":6,"n_cols":4,"rows_kept":6}
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[-0.117,100,0,17.9]
[-0.176,100,0,43.7]
[-0.257,99.73,0.27,74.8]
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{"sheet":"Fig3a","index":9,"n_rows":1002,"n_cols":4,"rows_kept":1002,"merged":[[0,0,0,1],[0,2,0,3]]}
["Initial",null,"After 1000-h stability test"]
["Potential (V) vs. RHE","Current density (A cm-2)","Potential (V) vs. RHE","Current density (A cm-2)"]
[0.14919,0.00187,0.24791,0.0024]
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["--","--",-0.34822,-0.2334]
["--","--",-0.34837,-0.2339]
["--","--",-0.3492,-0.234]

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["Cu2O/Cu",null,"CuO@Cu",null,"CuO@Cu-after1000h"]
["2θ (degree)","Intensity (arb. units)","2θ (degree)","Intensity (arb. units)","2θ (degree)","Intensity (arb. units)"]
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{"sheet":"Fig3c","index":11,"n_rows":253,"n_cols":6,"rows_kept":253,"merged":[[0,0,0,1],[0,2,0,3],[0,4,0,5]]}
["initial",null,"After CV activation",null,"After 1000 h"]
["Kinetic energy (eV)","Intensity (arb. units)","Kinetic energy (eV)","Intensity (arb. units)","Kinetic energy (eV)","Intensity (arb. units)"]
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[{"v":4000.122,"d":"4.00E+03"},{"v":0.000230906,"d":"2.31E-04"},4000.122,{"v":0.000418685,"d":"4.19E-04"},4000.122,1.06E-3,4000.122,0.00153,4000.122,0.00206,4000.122,0.00386,4000.122,0.0051,4000.122,0.00575,4000.122,0.00764,4000.122,0.01404,4000.122,-0.00279]

{"sheet":"Fig. 5b","index":20,"n_rows":16,"n_cols":5,"rows_kept":16}
["Fig. 5b"]
[null,"G / eV",null,null,"G / eV"]
["Coord","Cu(111)",null,"Coord","CuOx"]
["CH3CN+*",0,null,"CH3CN+*",0]
["*CH3CN",-0.21118,null,"*CH3CN",-0.07246]
["TS",0.69869,null,"*CH3CN+*H",-0.6208]
["*CH3CHN",-0.55579,null,"TS",-0.09297]
["TS",-0.03861,null,"*CH3CHN",-0.75499]
["*CH3CHNH",-1.23842,null,"TS",-0.14533]
["*CH3CHNH+*H",-1.71132,null,"*CH3CHNH",-1.29026]
["TS",-0.68214,null,"*CH3CHNH+H*",-1.8386]
["*CH3CH2NH",-1.4557,null,"TS",-1.06747]
["TS",-0.97066,null,"*CH3CH2NH",-1.88697]
["*CH3CH2NH2",-2.44096,null,"TS",-1.14293]
["CH3CH2NH2+*",-2.18829,null,"*CH3CH2NH2",-2.4766]
[{"$nulls":3},"CH3CH2NH2+*",-2.18829]

{"sheet":"FigS1a","index":21,"n_rows":802,"n_cols":6,"rows_kept":802,"merged":[[0,0,0,1],[0,2,0,3],[0,4,0,5]]}
["CuO@Cu-350",null,"CuO@Cu-450",null,"CuO@Cu-550"]
["Potential (V) vs. RHE","Current density (mA cm-2)","Potential (V) vs. RHE","Current density (mA cm-2)","Potential (V) vs. RHE","Current density (mA cm-2)"]
[0.05649,-1.47E-3,0.05649,-0.00178,0.05649,{"v":-6.69E-4,"d":"-6.69E-04"}]
[0.05548,-0.00146,0.05548,-0.00178,0.05548,{"v":-0.0006852,"d":"-6.85E-04"}]
[0.05444,-0.00143,0.05444,-0.00177,0.05444,{"v":-0.0006806,"d":"-6.81E-04"}]
[0.05337,-1.39E-3,0.05337,-1.74E-3,0.05337,{"v":-0.0006764,"d":"-6.76E-04"}]
[0.0523,-0.00136,0.0523,-1.72E-3,0.0523,{"v":-0.0006729,"d":"-6.73E-04"}]
[0.05126,-1.33E-3,0.05126,-1.67E-3,0.05126,{"v":-0.0006664,"d":"-6.66E-04"}]
[0.05019,-0.00129,0.05019,-1.66E-3,0.05019,{"v":-0.0006611,"d":"-6.61E-04"}]
[0.04913,-1.25E-3,0.04913,-1.67E-3,0.04913,{"v":-0.0006632,"d":"-6.63E-04"}]
[0.04811,-1.24E-3,0.04811,-1.66E-3,0.04811,{"v":-0.0006657,"d":"-6.66E-04"}]
[0.04709,-1.23E-3,0.04709,-0.00162,0.04709,{"v":-0.0006554,"d":"-6.55E-04"}]
[0.04606,-0.00121,0.04606,-0.00159,0.04606,{"v":-0.0006546,"d":"-6.55E-04"}]
[0.04503,-0.00119,0.04503,-1.56E-3,0.04503,{"v":-6.602E-4,"d":"-6.60E-04"}]
[0.044,-1.17E-3,0.044,-0.00155,0.044,{"v":-0.0006561,"d":"-6.56E-04"}]
[0.04297,-1.16E-3,0.04297,-0.00153,0.04297,{"v":-0.0006524,"d":"-6.52E-04"}]
[0.04197,-1.16E-3,0.04197,-1.56E-3,0.04197,{"v":-0.0006476,"d":"-6.48E-04"}]
[0.04094,-1.14E-3,0.04094,-1.57E-3,0.04094,{"v":-0.0006481,"d":"-6.48E-04"}]
[0.03992,-0.00113,0.03992,-1.57E-3,0.03992,{"v":-0.0006485,"d":"-6.49E-04"}]
[0.03893,-1.14E-3,0.03893,-0.00155,0.03893,{"v":-0.0006474,"d":"-6.47E-04"}]
[0.0379,-0.00112,0.0379,-0.00153,0.0379,{"v":-0.0006413,"d":"-6.41E-04"}]
[0.03688,-0.0011,0.03688,-0.00151,0.03688,{"v":-0.0006389,"d":"-6.39E-04"}]
[0.03585,-1.09E-3,0.03585,-1.5E-3,0.03585,{"v":-0.000636,"d":"-6.36E-04"}]
[0.03483,-1.08E-3,0.03483,-0.00152,0.03483,{"v":-0.0006349,"d":"-6.35E-04"}]
[0.03379,-0.00105,0.03379,-0.00152,0.03379,{"v":-0.0006312,"d":"-6.31E-04"}]
[0.03276,-0.00103,0.03276,-1.5E-3,0.03276,{"v":-0.0006306,"d":"-6.31E-04"}]
[0.03177,-0.00104,0.03177,-0.00153,0.03177,{"v":-0.0006294,"d":"-6.29E-04"}]
[0.03077,-0.00104,0.03077,-0.00151,0.03077,{"v":-0.000626,"d":"-6.26E-04"}]
[0.02977,-0.00104,0.02977,-0.00146,0.02977,{"v":-0.0006264,"d":"-6.26E-04"}]
[0.02874,-0.00102,0.02874,-0.00144,0.02874,{"v":-6.244E-4,"d":"-6.24E-04"}]
[0.02774,-0.00103,0.02774,-0.00146,0.02774,{"v":-0.0006275,"d":"-6.28E-04"}]
[0.02676,-0.00104,0.02676,-1.47E-3,0.02676,{"v":-6.265E-4,"d":"-6.27E-04"}]
[0.02576,-0.00103,0.02576,-0.00146,0.02576,{"v":-0.0006268,"d":"-6.27E-04"}]
[0.02471,-1.01E-3,0.02471,-0.00144,0.02471,{"v":-0.000625,"d":"-6.25E-04"}]
[0.02369,{"v":-0.0009927,"d":"-9.93E-04"},0.02369,-1.42E-3,0.02369,{"v":-6.29E-4,"d":"-6.29E-04"}]
[0.02267,{"v":-0.0009797,"d":"-9.80E-04"},0.02267,-1.41E-3,0.02267,{"v":-0.0006296,"d":"-6.30E-04"}]
[0.02164,{"v":-0.0009641,"d":"-9.64E-04"},0.02164,-0.00143,0.02164,{"v":-6.267E-4,"d":"-6.27E-04"}]
[0.02064,{"v":-0.000963,"d":"-9.63E-04"},0.02064,-0.00145,0.02064,{"v":-0.0006308,"d":"-6.31E-04"}]
[0.01964,{"v":-0.0009633,"d":"-9.63E-04"},0.01964,-1.4E-3,0.01964,{"v":-0.0006277,"d":"-6.28E-04"}]
[0.01862,{"v":-0.0009533,"d":"-9.53E-04"},0.01862,-1.42E-3,0.01862,{"v":-0.000626,"d":"-6.26E-04"}]
[0.01763,{"v":-0.0009573,"d":"-9.57E-04"},0.01763,-0.00138,0.01763,{"v":-0.0006229,"d":"-6.23E-04"}]
[0.01662,{"v":-0.0009524,"d":"-9.52E-04"},0.01662,-1.4E-3,0.01662,{"v":-0.0006193,"d":"-6.19E-04"}]
[0.0156,{"v":-0.0009438,"d":"-9.44E-04"},0.0156,-0.00137,0.0156,{"v":-0.0006181,"d":"-6.18E-04"}]
[0.01465,{"v":-0.0009685,"d":"-9.69E-04"},0.01465,-0.00138,0.01465,{"v":-0.0006162,"d":"-6.16E-04"}]
[0.01368,{"v":-0.0009866,"d":"-9.87E-04"},0.01368,-1.4E-3,0.01368,{"v":-0.0006195,"d":"-6.20E-04"}]
[0.01265,{"v":-0.0009731,"d":"-9.73E-04"},0.01265,-1.41E-3,0.01265,{"v":-0.0006256,"d":"-6.26E-04"}]
[0.01165,{"v":-0.00097,"d":"-9.70E-04"},0.01165,-1.4E-3,0.01165,{"v":-0.000624,"d":"-6.24E-04"}]
[0.0107,-1E-3,0.0107,-1.41E-3,0.0107,{"v":-0.0006209,"d":"-6.21E-04"}]
[0.00967,{"v":-0.0009849,"d":"-9.85E-04"},0.00967,-1.4E-3,0.00967,{"v":-0.0006213,"d":"-6.21E-04"}]
[8.6E-3,{"v":-0.0009388,"d":"-9.39E-04"},8.6E-3,-1.39E-3,8.6E-3,{"v":-0.0006261,"d":"-6.26E-04"}]
[0.00758,{"v":-0.0009265,"d":"-9.27E-04"},0.00758,-0.00138,0.00758,{"v":-0.0006214,"d":"-6.21E-04"}]
[0.00655,{"v":-0.0009111,"d":"-9.11E-04"},0.00655,-0.00137,0.00655,{"v":-0.0006238,"d":"-6.24E-04"}]
[0.00559,{"v":-0.0009355,"d":"-9.36E-04"},0.00559,-1.33E-3,0.00559,{"v":-0.0006175,"d":"-6.18E-04"}]
[0.0046,{"v":-0.000943,"d":"-9.43E-04"},0.0046,-1.34E-3,0.0046,{"v":-0.0006111,"d":"-6.11E-04"}]
[3.63E-3,{"v":-0.0009564,"d":"-9.56E-04"},3.63E-3,-0.00135,3.63E-3,{"v":-0.0006136,"d":"-6.14E-04"}]
[2.63E-3,{"v":-0.0009596,"d":"-9.60E-04"},2.63E-3,-1.34E-3,2.63E-3,{"v":-0.0006125,"d":"-6.13E-04"}]
[1.57E-3,{"v":-0.0009264,"d":"-9.26E-04"},1.57E-3,-0.00136,1.57E-3,{"v":-0.0006113,"d":"-6.11E-04"}]
[{"v":5.4955E-4,"d":"5.50E-04"},{"v":-0.0009115,"d":"-9.12E-04"},{"v":5.4955E-4,"d":"5.50E-04"},-0.00137,{"v":5.4955E-4,"d":"5.50E-04"},{"v":-0.0006139,"d":"-6.14E-04"}]
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[-1.47E-3,{"v":-0.0009005,"d":"-9.01E-04"},-1.47E-3,-0.00136,-1.47E-3,{"v":-0.0006136,"d":"-6.14E-04"}]
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[-0.0055,{"v":-0.0008835,"d":"-8.84E-04"},-0.0055,-1.33E-3,-0.0055,{"v":-0.0006129,"d":"-6.13E-04"}]
[-0.00649,{"v":-0.0008867,"d":"-8.87E-04"},-0.00649,-1.33E-3,-0.00649,{"v":-0.0006138,"d":"-6.14E-04"}]
[-0.0075,{"v":-0.0008841,"d":"-8.84E-04"},-0.0075,-1.33E-3,-0.0075,{"v":-0.0006101,"d":"-6.10E-04"}]
[-0.00849,{"v":-0.0008862,"d":"-8.86E-04"},-0.00849,-1.32E-3,-0.00849,{"v":-0.0006122,"d":"-6.12E-04"}]
[-0.00949,{"v":-0.0008875,"d":"-8.88E-04"},-0.00949,-1.32E-3,-0.00949,{"v":-0.0006132,"d":"-6.13E-04"}]
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[-0.01248,{"v":-0.0008912,"d":"-8.91E-04"},-0.01248,-1.33E-3,-0.01248,{"v":-0.0006174,"d":"-6.17E-04"}]
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[-0.01455,{"v":-0.0008539,"d":"-8.54E-04"},-0.01455,-0.00136,-0.01455,{"v":-6.177E-4,"d":"-6.18E-04"}]
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{"sheet":"FigS1b","index":22,"n_rows":6,"n_cols":4,"rows_kept":6}
["Potential (V) vs. RHE","FE(EA)","FE(H2)","Current density (mA cm-2)"]
[-0.261,100,0,5]
[-0.342,99.65,0.35,18.7]
[-0.406,99.95,0.05,44.5]
[-0.423,99.09,0.91,89.4]
[-0.462,93.99,6.01,218.9]

{"sheet":"FigS1c","index":23,"n_rows":7,"n_cols":4,"rows_kept":7}
["Potential (V) vs. RHE","FE(EA)","FE(H2)","Current density (mA cm-2)"]
[-0.251,99.88,0,11.1]
[-0.315,101.41,0.25,38.4]
[-0.37,99.86,0.42,70.8]
[-0.4,98.67,0.83,120.6]
[-0.44,98.16,1.87,160.2]
[-0.456,95.32,4.01,223.6]

{"sheet":"FigS1d","index":24,"n_rows":7,"n_cols":4,"rows_kept":7}
["Potential (V) vs. RHE","FE(EA)","FE(H2)","Current density (mA cm-2)"]
[-0.254,99.54,0.46,10.3]
[-0.326,99.04,0.96,30.7]
[-0.382,93.75,6.25,61.8]
[-0.412,82.2,17.8,111.9]
[-0.423,73.59,26.41,174.4]
[-0.442,65.83,34.17,233.4]

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["Potential (V) vs. RHE","Current density (mA cm-2)"]
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[0.23,0.00409]
[0.229,0.00339]
[0.228,0.00269]
[0.227,2.14E-3]
[0.226,0.00168]
[0.225,1.14E-3]
[0.224,{"v":0.0007274,"d":"7.27E-04"}]
[0.223,{"v":0.0003639,"d":"3.64E-04"}]
[0.222,{"v":-8.118e-05,"d":"-8.12E-05"}]
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[-0.022,-0.00193]
[-0.021,-1.83E-3]
[-0.02,-1.82E-3]
[-0.019,-0.0017]
[-0.018,-0.00163]
[-0.017,-0.00163]
[-0.016,-1.5E-3]
[-0.015,-0.00144]
[-0.014,-0.00144]
[-0.013,-1.33E-3]
[-0.012,-0.00128]
[-0.011,-0.00127]
[-0.01,-1.15E-3]
[-0.009,-0.00105]
[-0.008,-0.00104]
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[-0.004,{"v":-0.0006984,"d":"-6.98E-04"}]
[-0.003,{"v":-0.0006253,"d":"-6.25E-04"}]
[-2E-3,{"v":-0.0006095,"d":"-6.10E-04"}]
[-1E-3,{"v":-0.000481,"d":"-4.81E-04"}]
[0,{"v":-0.0004128,"d":"-4.13E-04"}]
[1E-3,{"v":-0.0004106,"d":"-4.11E-04"}]
[2E-3,{"v":-0.0002773,"d":"-2.77E-04"}]
[0.003,{"v":-0.0002146,"d":"-2.15E-04"}]
[0.004,{"v":-0.0002101,"d":"-2.10E-04"}]
[0.005,{"v":-9.169e-05,"d":"-9.17E-05"}]
[0.006,{"v":-2.345e-05,"d":"-2.35E-05"}]
[0.007,{"v":5.106e-07,"d":"5.11E-07"}]
[0.008,{"v":0.0001264,"d":"1.26E-04"}]
[0.009,{"v":0.00021,"d":"2.10E-04"}]
[0.01,{"v":0.0002155,"d":"2.16E-04"}]
[0.011,{"v":3.458E-4,"d":"3.46E-04"}]
[0.012,{"v":0.0004254,"d":"4.25E-04"}]
[0.013,{"v":0.0004423,"d":"4.42E-04"}]
[0.014,{"v":0.0005791,"d":"5.79E-04"}]
[0.015,{"v":0.0006145,"d":"6.15E-04"}]
[0.016,{"v":0.000615,"d":"6.15E-04"}]
[0.017,{"v":0.0007296,"d":"7.30E-04"}]
[0.018,{"v":0.0007638,"d":"7.64E-04"}]
[0.019,{"v":7.896E-4,"d":"7.90E-04"}]
[0.02,{"v":0.0009285,"d":"9.29E-04"}]
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[0.035,1.9E-3]
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[0.038,0.0021]
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[0.057,0.00312]
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[0.061,0.00339]
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[0.063,0.00345]
[0.064,0.00352]
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[0.077,0.00407]
[0.078,0.00402]
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[0.081,0.0041]
[0.082,4.13E-3]
[0.083,0.0042]
[0.084,0.00416]
[0.085,0.00419]
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[0.087,0.00423]
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[0.169,0.00469]
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[0.172,0.00475]
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[0.175,4.79E-3]
[0.176,0.00474]
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[0.178,0.00484]
[0.179,0.0048]
[0.18,0.00483]
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[0.184,0.00495]
[0.185,0.0049]
[0.186,0.00494]
[0.187,0.00502]
[0.188,0.00497]
[0.189,0.00504]
[0.19,0.0051]
[0.191,0.00506]
[0.192,5.13E-3]
[0.193,0.0052]
[0.194,0.00516]
[0.195,0.0052]
[0.196,0.00526]
[0.197,0.00522]
[0.198,0.00525]
[0.199,0.00534]
[0.2,0.00531]
[0.201,0.00535]
[0.202,0.00543]
[0.203,0.00539]
[0.204,5.45E-3]
[0.205,0.00553]
[0.206,0.00551]
[0.207,0.00556]
[0.208,5.62E-3]
[0.209,0.0056]
[0.21,0.00566]
[0.211,0.00573]
[0.212,0.0057]
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[0.219,0.00602]
[0.22,0.00607]
[0.221,0.00605]
[0.222,0.00617]
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[0.225,0.00629]
[0.226,0.00634]
[0.227,0.00632]
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[0.23,6.43E-3]
[0.231,0.00654]
[0.231,0.0048]

{"sheet":"FigS2b","index":26,"n_rows":4002,"n_cols":2,"rows_kept":4002}
["Potential (V) vs. RHE","Current density (mA cm-2)"]
[0.231,0.00883]
[0.23,0.00881]
[0.229,0.00888]
[0.228,0.00898]
[0.227,0.00901]
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[0.222,0.00631]
[0.221,5.64E-3]
[0.22,0.00509]
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[0.217,0.0035]
[0.216,3.15E-3]
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[0.213,0.00209]
[0.212,1.83E-3]
[0.211,1.57E-3]
[0.21,1.25E-3]
[0.209,{"v":9.391E-4,"d":"9.39E-04"}]
[0.208,{"v":0.0007312,"d":"7.31E-04"}]
[0.207,{"v":0.0005499,"d":"5.50E-04"}]
[0.206,{"v":0.0002994,"d":"2.99E-04"}]
[0.205,{"v":3.065E-5,"d":"3.07E-05"}]
[0.204,{"v":-0.0001541,"d":"-1.54E-04"}]
[0.203,{"v":-0.000279,"d":"-2.79E-04"}]
[0.202,{"v":-0.0004496,"d":"-4.50E-04"}]
[0.201,{"v":-0.0006777,"d":"-6.78E-04"}]
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{"sheet":"FigS4","index":28,"n_rows":1002,"n_cols":4,"rows_kept":1002,"merged":[[0,0,0,1],[0,2,0,3]]}
["1 M NaOH + 12wt% MeCN",null,"1 M NaOH"]
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{"sheet":"FigS5","index":29,"n_rows":1002,"n_cols":6,"rows_kept":1002,"merged":[[0,0,0,1],[0,2,0,3],[0,4,0,5]]}
["Cu foam",null,"CuO@Cu",null,"OD-Cu"]
["Potential (V) vs. RHE","Current density (mA cm-2)","Potential (V) vs. RHE","Current density (mA cm-2)","Potential (V) vs. RHE","Current density (mA cm-2)"]
[0.037,{"v":-1.917E-4,"d":"-1.92E-04"},0.13749,0.00187,0.231,{"v":0.0007671,"d":"7.67E-04"}]
[0.036,{"v":-2.065E-4,"d":"-2.07E-04"},0.1364,0.00152,0.22959,{"v":0.0004558,"d":"4.56E-04"}]
[0.035,{"v":-2.117E-4,"d":"-2.12E-04"},0.13533,1.25E-3,0.22838,{"v":0.000289,"d":"2.89E-04"}]
[0.034,{"v":-0.0002093,"d":"-2.09E-04"},0.13427,0.00104,0.22722,{"v":0.0001723,"d":"1.72E-04"}]
[0.033,{"v":-2.119E-4,"d":"-2.12E-04"},0.13323,{"v":0.0008708,"d":"8.71E-04"},0.22613,{"v":9.78e-05,"d":"9.78E-05"}]
[0.032,{"v":-0.0002124,"d":"-2.12E-04"},0.13219,{"v":0.0007268,"d":"7.27E-04"},0.22505,{"v":4.006e-05,"d":"4.01E-05"}]
[0.031,{"v":-0.0002188,"d":"-2.19E-04"},0.13116,{"v":0.0006052,"d":"6.05E-04"},0.22397,{"v":-2.16E-5,"d":"-2.16E-05"}]
[0.03,{"v":-0.000218,"d":"-2.18E-04"},0.13013,{"v":0.0005034,"d":"5.03E-04"},0.2229,{"v":-7.973e-05,"d":"-7.97E-05"}]
[0.029,{"v":-0.0002171,"d":"-2.17E-04"},0.12911,{"v":0.0004114,"d":"4.11E-04"},0.22183,{"v":-0.0001274,"d":"-1.27E-04"}]
[0.028,{"v":-0.000217,"d":"-2.17E-04"},0.12809,{"v":3.321E-4,"d":"3.32E-04"},0.2208,{"v":-0.0001575,"d":"-1.58E-04"}]
[0.027,{"v":-0.0002212,"d":"-2.21E-04"},0.12707,{"v":2.586E-4,"d":"2.59E-04"},0.21976,{"v":-0.0001843,"d":"-1.84E-04"}]
[0.026,{"v":-0.000221,"d":"-2.21E-04"},0.12605,{"v":0.0001913,"d":"1.91E-04"},0.21872,{"v":-0.0002172,"d":"-2.17E-04"}]
[0.025,{"v":-2.196E-4,"d":"-2.20E-04"},0.12503,{"v":0.0001286,"d":"1.29E-04"},0.21767,{"v":-0.000254,"d":"-2.54E-04"}]
[0.024,{"v":-2.187E-4,"d":"-2.19E-04"},0.12402,{"v":6.52e-05,"d":"6.52E-05"},0.21662,{"v":-0.0002891,"d":"-2.89E-04"}]
[0.023,{"v":-2.243E-4,"d":"-2.24E-04"},0.123,{"v":1.155E-5,"d":"1.16E-05"},0.21559,{"v":-0.0003151,"d":"-3.15E-04"}]
[0.022,{"v":-0.0002282,"d":"-2.28E-04"},0.12199,{"v":-3.653e-05,"d":"-3.65E-05"},0.21457,{"v":-0.000332,"d":"-3.32E-04"}]
[0.021,{"v":-0.000228,"d":"-2.28E-04"},0.12098,{"v":-8.185e-05,"d":"-8.19E-05"},0.21355,{"v":-3.457E-4,"d":"-3.46E-04"}]
[0.02,{"v":-0.0002305,"d":"-2.31E-04"},0.11997,{"v":-1.193E-4,"d":"-1.19E-04"},0.21252,{"v":-0.0003668,"d":"-3.67E-04"}]
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{"sheet":"FigS7a","index":30,"n_rows":902,"n_cols":4,"rows_kept":902,"merged":[[0,0,0,1],[0,2,0,3]]}
["CuO@Cu",null,"CuO NP"]
["Potential (V) vs. RHE","Current density (A cm-2)","Potential (V) vs. RHE","Current density (A cm-2)"]
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{"sheet":"FigS7b","index":31,"n_rows":6,"n_cols":4,"rows_kept":6}
["Potential (V) vs. RHE","FE(EA)","FE(H2)","Current density (mA cm-2)"]
[-0.15,96,4,-0.005]
[-0.2,91.36,8.64,-0.025]
[-0.25,89.33,10.67,-0.05033]
[-0.3,82.54,17.46,-0.0894]
[-0.325,81.33,18.67,-0.12036]

{"sheet":"FigS8","index":32,"n_rows":6,"n_cols":4,"rows_kept":6}
["Potential (V) vs. RHE","FE(EA)","FE(H2)","Current density (mA cm-2)"]
[-0.22,97.3,2.7,13]
[-0.33,95.4,4.6,36]
[-0.38,89.3,10.7,56]
[-0.42,89.1,10.9,76]
[-0.49,84.6,15.4,102]

{"sheet":"FigS9","index":33,"n_rows":6,"n_cols":4,"rows_kept":6}
["Potential (V) vs. RHE","FE(EA)","FE(H2)","Current density (mA cm-2)"]
[-0.314,55.4,44.6,10]
[-0.4,50.3,49.7,28.4]
[-0.435,44.3,55.7,39.1]
[-0.479,32.1,67.9,52.7]
[-0.589,28.9,71.1,81.6]

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["1M NaOH",null,"0.5M NaOH + 0.25M Na2SO4",null," 0.1M NaOH + 0.45M Na2SO4",null,"0.5M Na2SO4"]
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[-0.36475,null,-0.36475,null,-0.36475,null,-0.36475,-0.2515]
[-0.3653,null,-0.3653,null,-0.3653,null,-0.3653,-0.2518]
[-0.366,null,-0.366,null,-0.366,null,-0.366,-0.252]
[-0.3664,null,-0.3664,null,-0.3664,null,-0.3664,-0.2524]
[-0.36665,null,-0.36665,null,-0.36665,null,-0.36665,-0.2529]
[-0.3669,null,-0.3669,null,-0.3669,null,-0.3669,-0.2534]

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["1M NaOH",null,"0.5M NaOH + 0.25M Na2SO4",null," 0.1M NaOH + 0.45M Na2SO4",null,"0.5M Na2SO4"]
["Potential (V) vs. RHE","FE(EA)","Potential (V) vs. RHE","FE(EA)","Potential (V) vs. RHE","FE(EA)","Potential (V) vs. RHE","FE(EA)"]
[-0.117,100,-0.153,83,-0.209,72,-0.21,31.11]
[-0.176,100,-0.212,76,-0.225,68,-0.249,15.33]
[-0.257,99.73,-0.279,70,-0.301,63,-0.28,10.33]
[-0.314,99.12,-0.305,66,-0.315,60,-0.31,7.23]
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["8 % acetonitrile",null,"12 % acetonitrile",null,"16 % acetonitrile"]
["Potential (V) vs. RHE","Current density (mA cm-2)","Potential (V) vs. RHE","Current density (mA cm-2)","Potential (V) vs. RHE","Current density (mA cm-2)"]
[0.0558,-1.06E-3,0.06329,-0.00546,0.05574,-0.00102]
[0.05484,-1.08E-3,0.06208,-0.00534,0.05478,-0.00105]
[0.05382,-1.07E-3,0.06084,-0.0052,0.05376,-0.00103]
[0.05283,-1.07E-3,0.05965,-0.00509,0.05276,-0.00103]
[0.05182,-1.07E-3,0.05831,-0.00489,0.05174,-0.00102]
[0.05081,-1.06E-3,0.05707,-0.00475,0.05074,-0.00102]
[0.0498,-1.06E-3,0.05583,-0.0046,0.04974,-0.00102]
[0.0488,-1.06E-3,0.05466,-0.00451,0.04871,-1.01E-3]
[0.04778,-0.00105,0.05345,-0.00438,0.04772,-1.01E-3]
[0.04677,-0.00104,0.05232,-4.3E-3,0.04671,-1.01E-3]
[0.04576,-0.00104,0.05108,-0.00417,0.0457,{"v":-0.0009982,"d":"-9.98E-04"}]
[0.04476,-0.00104,0.04992,-0.00407,0.0447,-1E-3]
[0.04377,-0.00104,0.04868,-0.00393,0.04369,{"v":-0.0009919,"d":"-9.92E-04"}]
[0.04276,-0.00104,0.04736,-0.00374,0.04268,{"v":-0.000989,"d":"-9.89E-04"}]
[0.04175,-0.00103,0.04624,-0.00367,0.04166,{"v":-0.0009766,"d":"-9.77E-04"}]
[0.04076,-0.00103,0.04516,-3.62E-3,0.04067,{"v":-0.0009818,"d":"-9.82E-04"}]
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[0.03676,-0.00103,0.0406,-3.3E-3,0.03668,{"v":-0.0009876,"d":"-9.88E-04"}]
[0.03573,-0.00102,0.0395,-0.00323,0.03567,{"v":-0.0009842,"d":"-9.84E-04"}]
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[0.03174,-0.00102,0.03525,-0.00309,0.03165,{"v":-0.0009725,"d":"-9.73E-04"}]
[0.03071,-1.01E-3,0.03422,-0.00307,0.03064,{"v":-0.000962,"d":"-9.62E-04"}]
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[null,"8 wt% acetonitrile",null,"12 wt% acetonitrile",null,"16 wt% acetonitrile"]
["Potential (V) vs. RHE","FE(EA)","FE(H2)","FE(EA)","FE(H2)","FE(EA)","FE(H2)"]
[-0.254,100,0,99.88,0,99.54,0.46]
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{"sheet":"FigS16a","index":38,"n_rows":468,"n_cols":4,"rows_kept":468,"merged":[[0,0,0,1]]}
["OCP",null,"CV cycling","CA test (after 1 h)"]
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["OCP",null,"CV cycling","CA test (after 1 h)"]
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{"sheet":"FigS18","index":40,"n_rows":102,"n_cols":2,"rows_kept":102}
["Potential (V) vs. RHE","log|j| (mA cm-2)"]
[-0.0519,-1.99311]
[-0.05234,-1.9897]
[-0.05282,-1.98801]
[-0.05325,-1.9838]
[-0.05373,-1.98255]
[-0.05417,-1.9784]
[-0.05457,-1.97224]
[-0.05498,-1.96658]
[-0.05545,-1.96457]
[-0.05588,-1.96059]
[-0.05634,-1.95782]
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[-0.05764,-1.94615]
[-0.0581,-1.94348]
[-0.05853,-1.9393]
[-0.05899,-1.93704]
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[-0.05988,-1.9307]
[-0.06027,-1.92445]
[-0.06067,-1.91937]
[-0.06112,-1.9165]
[-0.06157,-1.91364]
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[-0.06334,-1.90101]
[-0.06384,-1.90136]
[-0.06427,-1.89757]
[-0.06464,-1.89076]
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[-0.0655,-1.88372]
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[-0.06968,-1.84345]
[-0.07008,-1.83893]
[-0.07053,-1.83654]
[-0.07102,-1.83594]
[-0.07139,-1.83033]
[-0.0718,-1.82594]
[-0.07219,-1.82131]
[-0.07258,-1.81645]
[-0.07302,-1.81389]
[-0.07345,-1.81079]
[-0.07386,-1.80688]
[-0.07424,-1.80189]
[-0.07424,-1.80189]
[-0.07501,-1.7921]
[-0.07543,-1.78888]
[-0.07585,-1.78569]
[-0.07627,-1.78225]
[-0.07666,-1.7778]
[-0.07707,-1.77443]
[-0.07746,-1.76981]
[-0.07781,-1.76397]
[-0.07823,-1.76095]
[-0.07864,-1.75771]
[-0.07903,-1.7535]
[-0.07945,-1.75031]
[-0.07985,-1.74666]
[-0.08024,-1.74256]
[-0.08061,-1.73755]
[-0.08101,-1.73424]
[-0.0814,-1.73025]
[-0.08181,-1.727]
[-0.08221,-1.72331]
[-0.0826,-1.71942]
[-0.083,-1.71602]
[-0.0834,-1.71242]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]
["--","--"]

{"sheet":"Fig. S23","index":41,"n_rows":10,"n_cols":13,"rows_kept":10}
["Fig. S23"]
[null,"G / eV",null,"G / eV",null,"G / eV",null,null,"G / eV",null,"G / eV",null,"G / eV"]
["Coord","Cu(111)","Coord","Cu(111)","Coord","Cu(111)",null,"Coord","CuOx","Coord","CuOx","Coord","CuOx"]
["CH3CN+*",0,{"$nulls":5},"CH3CN+*",0]
["*CH3CN",-0.21118,{"$nulls":5},"*CH3CN",-0.07246]
["*CH3CHN",-0.15579,"*CH3CNH",0.05171,{"$nulls":3},"*CH3CHN",-0.35499,"*CH3CNH",-0.34353]
["*CH3CHNH",-0.43842,"*CH3CH2N",-0.04048,"*CH3CNH2",-0.05313,null,"*CH3CHNH",-0.49026,"*CH3CH2N",-0.0814,"*CH3CNH2",-0.19751]
["*CH3CH2NH",-0.2557,"*CH3CHNH2",-0.05107,{"$nulls":3},"*CH3CH2NH",-0.68697,"*CH3CHNH2",-0.19496]
["*CH3CH2NH2",-0.84096,{"$nulls":5},"*CH3CH2NH2",-0.8766]
["CH3CH2NH2+*",-0.58829,{"$nulls":5},"CH3CH2NH2+*",-0.58829]

{"sheet":"Fig. S24","index":42,"n_rows":18,"n_cols":6,"rows_kept":18}
["Fig. S24"]
[null,"H2O path","G / eV",null,"surface pathway","G / eV"]
[null,"Coord","Cu(111)",null,"Coord","Cu(111)"]
[null,"CH3CN+*",0,null,"CH3CN+*",0]
[null,"*CH3CN",-0.21118,null,"*CH3CN",-0.21118]
[null,"TS",0.69869,null,"*CH3CN+*H",-0.68408]
[null,"*CH3CHN",-0.55579,null,"TS",0.23663]
[null,"TS",-0.03861,null,"*CH3CHN",-0.55579]
[null,"*CH3CHNH",-1.23842,null,"*CH3CHN+*H",-1.0287]
[null,"TS",0.24951,null,"TS",-3.96E-3]
[null,"*CH3CH2NH",-1.4557,null,"*CH3CHNH",-1.23842]
[null,"TS",-0.97066,null,"*CH3CHNH+*H",-1.71132]
[null,"*CH3CH2NH2",-2.44096,null,"TS",-0.68214]
[null,"CH3CH2NH2+*",-2.18829,null,"*CH3CH2NH",-1.4557]
[{"$nulls":4},"*CH3CH2NH+*H",-1.9286]
[{"$nulls":4},"TS",-0.81684]
[{"$nulls":4},"*CH3CH2NH2",-2.44096]
[{"$nulls":4},"CH3CH2NH2+*",-2.18829]

{"sheet":"Fig. S25","index":43,"n_rows":18,"n_cols":6,"rows_kept":18}
["Fig. S25"]
[null,"H2O path","G / eV",null,"surface pathway","G / eV"]
[null,"Coord","CuOx",null,"Coord","CuOx"]
[null,"CH3CN+*",0,null,"CH3CN+*",0]
[null,"*CH3CN",-0.07246,null,"*CH3CN",-0.07246]
[null,"TS",0.94095,null,"*CH3CN+*H",-0.6208]
[null,"*CH3CHN",-0.75499,null,"TS",-0.09297]
[null,"TS",-0.14533,null,"*CH3CHN",-0.75499]
[null,"*CH3CHNH",-1.29026,null,"*CH3CHN+*H",-1.30333]
[null,"TS",-0.22121,null,"TS",-0.52924]
[null,"*CH3CH2NH",-1.88697,null,"*CH3CHNH",-1.29026]
[null,"TS",-1.14293,null,"*CH3CHNH+*H",-1.8386]
[null,"*CH3CH2NH2",-2.4766,null,"TS",-1.06747]
[null,"CH3CH2NH2+*",-2.18829,null,"*CH3CH2NH",-1.88697]
[{"$nulls":4},"*CH3CH2NH+*H",-2.43531]
[{"$nulls":4},"TS",-1.20162]
[{"$nulls":4},"*CH3CH2NH2",-2.4766]
[{"$nulls":4},"CH3CH2NH2+*",-2.18829]

{"sheet":"Fig. S26","index":44,"n_rows":4,"n_cols":3,"rows_kept":4}
["Fig. S26"]
[null,"ΔG / eV","ΔG / eV"]
[null,"Cu(111)","CuOx"]
["H*",-0.0729032100000424,-0.14833951999997197]